CUED Publications database

Ultrafast Photophysics of Single-Walled Carbon Nanotubes

Soavi, G and Scotognella, F and Lanzani, G and Cerullo, G (2016) Ultrafast Photophysics of Single-Walled Carbon Nanotubes. Advanced Optical Materials, 4. pp. 1670-1688.

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Abstract

© 2016 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim Single-walled carbon nanotubes (SWNTs) are nanocylinders obtained by wrapping one layer of graphene; due to their very high aspect ratio, they are the prototypical quantum confined one-dimensional systems. The unique mechanical, electronic, and optical properties of SWNTs open up transversal application possibilities in many fields of science and technology, with particular emphasis on optoelectronics and photonics. A prerequisite for many of these applications is a thorough understanding of the nature and dynamics of their elementary excitations. This review aims at summarizing the current understanding of the ultrafast photophysics of SWNTs, based on two decades of experimental investigations. After discussing the morphological and electronic properties of SWNTs and introducing the different photogenerated species, we will briefly describe the ultrafast spectroscopic techniques most commonly used for their characterization. Finally, we present the experimental evidence that has led to establish the nature (singlet and triplet excitons, bi-excitons, trions, and free charges) and the relaxation pathways of photoexcitations in SWNTs.

Item Type: Article
Subjects: UNSPECIFIED
Divisions: Div B > Electronics, Power & Energy Conversion
Depositing User: Cron Job
Date Deposited: 17 Jul 2017 19:06
Last Modified: 26 Oct 2017 01:54
DOI: